a. by chance
Esta droga se descubrió de casualidad, mientras se investigaban los efectos de otra sustancia.This drug was discovered by chance, while the effects of other substance were being studied.
b. by accident
Cada tanto, nos encontramos de casualidad cuando estamos esperando el tren.Now and then, we meet by accident while we're waiting for the train.
De casualidad, ¿sabes cómo se llama el nuevo contador?Do you know what the new accountant's name is by any chance?
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